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Driven-Dissipative Phase Separation in Free-Space Atomic Ensembles

  • D. Goncalves*
  • , L. Bombieri
  • , G. Ferioli
  • , S. Pancaldi
  • , I. Ferrier-Barbut
  • , A. Browaeys
  • , E. Shahmoon
  • , D. E. Chang
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

Abstract

The driven Dicke model, wherein an ensemble of atoms is driven by an external field and undergoes collective spontaneous emission due to coupling to a leaky cavity mode, is a paradigmatic example of a system exhibiting a driven-dissipative phase transition as a function of driving strength. Recently, a similar phenomenon was experimentally observed, not in a cavity setting, but rather in a free-space atomic ensemble. The reason why similar behavior should emerge in free space is not obvious, as the system interacts with a continuum of optical modes, which encodes light-propagation effects. Here, we present and solve a simple model to explain the behavior of the free-space system, based on the one-dimensional Maxwell-Bloch equations. On one hand, we show that a free-space ensemble at a low optical depth can exhibit similar behavior as the cavity system, as spatial propagation effects are negligible. On the other hand, in the thermodynamic limit of large atom number, we show that certain observables such as the transmittance or the atomic excited population exhibit nonanalytic behavior as a function of the driving intensity, reminiscent of a phase transition. However, a closer analysis reveals that the atomic properties are highly inhomogeneous in space, and based on this we argue that the free-space system does not undergo a phase transition but rather a "phase separation,"roughly speaking, between saturated and unsaturated regions.

Original languageEnglish
Article number020303
JournalPRX Quantum
Volume6
Issue number2
DOIs
Publication statusPublished - Apr 2025

Funding

The authors acknowledge stimulating discussions with Fernando de Iemini, Jamir Marino, Francis Robicheaux, and Ana Maria Rey. D.G. acknowledges support from the Secretaria d’Universitats i Recerca de la Generalitat de Catalunya and the European Social Fund (2020 FI B 00196). L.B. acknowledges support from the European Union’s Horizon Europe research and innovation program under Grant Agreement No. 101113690 (PASQuanS2.1). E.S. acknowledges support from the Israel Science Foundation (ISF), the Center for New Scientists at the Weizmann Institute of Science, and the Council for Higher Education (Israel). D.E.C. acknowledges support from the European Union, under European Research Council European Research Council Grant Agreement No. 101002107 (NEWSPIN), FET-Open Grant Agreement No. 899275 (DAALI) and EIC Pathfinder Grant No. 101115420 (PANDA); the Government of Spain under Severo Ochoa Grant CEX2019-000910-S (MCIN/AEI/10.13039/501100011033); Generalitat de Catalunya (CERCA Program and AGAUR Project No. 2021 SGR 01442); Fundació Cellex, and Fundació Mir-Puig. This work is also supported by the Agence Nationale de la Recherche (ANR-22-PETQ-0004 France 2030, Project QuBitAF), and the European Research Council (Advanced Grant No. 101018511-ATARAXIA) and the Horizon Europe Programme HORIZON-CL4-2022-QUANTUM-02-SGA via the Project 101113690 (PASQuanS2.1).

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials
  • General Computer Science
  • Mathematical Physics
  • General Physics and Astronomy
  • Applied Mathematics
  • Electrical and Electronic Engineering

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